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Answer: TENSEST
TENSEST is a crossword puzzle answer that we have spotted 19 times.
Most wound up
Stretched to the limit
Most uptight
Least loose
Most likely to crack
Least relaxed
Most volatile
Most rigid
Most edgy
Having the least give
Most suspenseful
Superlatively suspenseful
Least lax
Most nail-biting
Most high-strung
Most likely to snap
Most gripping
Most charged
Most likely to snap, say